If the blocks are moving as shown in the figure the relation between a1, a2 and a3 will be
2a1+2a2+a3 = 0
2a1-2a2+a3 = 0
2a1-2a2-a3 = 0
2a2-2a1 +a3 = 0
From pulley (3)
a2 = 2a1-a32
2a2 = 2a1-a3